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Título: | Could an efficient WGS catalyst be useful in the CO-PrOx reaction? |
Autor: | Reina, T.R. CSIC ORCID; Papadopoulos, E.; Palma, Sergio; Ivanova, Svetlana CSIC ORCID; Centeno, Miguel Ángel CSIC ORCID; Ioannides, T.; Odriozola, José Antonio CSIC ORCID | Palabras clave: | PrOx Iron oxide Cerium oxide Gold catalysts H2 clean-up. |
Fecha de publicación: | 2014 | Editor: | Elsevier | Citación: | Applied Catalysis B: Environmental 150-151: 554- 563 (2014) | Resumen: | This work presents an evaluation of a high performance series of water gas shift (WGS) catalysts in the preferential CO oxidation reaction (PrOx) in order to examine the applicability of the same catalyst for both processes as a first step for coupling both reactions in a single process. Gold based catalysts are applied in an extensive study of the CO-PrOx reaction parameters, such as λ, WHSV, CO concentration and [H2O]/[CO2] ratio in order to obtain the best activity/selectivity balance. CO and H2 oxidation reactions were treated separately in order to establish the degree of CO/H2 oxidation competition. Additionally the catalysts behavior in the CO-PrOx parallel reactions such a WGS and RWGS have been also carried out to analyze their effect on product composition. © 2014 Elsevier B.V. | URI: | http://hdl.handle.net/10261/102015 | DOI: | 10.1016/j.apcatb.2014.01.001 | Identificadores: | doi: 10.1016/j.apcatb.2014.01.001 issn: 0926-3373 |
Aparece en las colecciones: | (ICMS) Artículos |
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manuscript revised_highlighted_2.pdf | 421,62 kB | Adobe PDF | Visualizar/Abrir |
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